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In this study, we focused on the amplification process of superfluorescence, which has been the subject of very few previous reports. We designed an original experiment that combined two types of lasers, a pulsed laser and a continuous wave laser, and demonstrated that the instantaneous light intensity of a continuous wave laser can be amplified by seven orders of magnitude by superfluorescence.
Attention to results
The paper was published in the online version of Physical Review Letters, a globally renowned journal in the field of physics, on Monday, February 12, 2024, having succeeded in demonstrating a new light amplification process that utilizes the atomic synchronization phenomenon known as superfluorescence, a well-known phenomenon in quantum mechanics.
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Assistant Professor Kenta Kitano
Faculty of Science and Engineering, Department of Physical Sciences
Graduated from the Department of Mathematics, Faculty of Science, Kyoto University. After working for a general company, he encountered quantum mechanics and was fascinated by it, so he enrolled in the Department of Chemistry, Graduate School of Science, Kyoto University, where he completed his master's course. He then completed his doctoral course in Structural Molecular Science, Graduate School of Physical Sciences, SOKENDAI (The Graduate University for Advanced Studies). He is currently employed in the Department of Physical Sciences, Faculty of Science and Engineering, Kyoto University (formerly the Department of Physics and Mathematics at the time of assuming his post) in April 2015. His fields of expertise are quantum mechanics, lasers, and atoms and molecules. He has been conducting research into superfluorescence since around 2016.
By using superfluorescence, the intensity of laser light has been increased by approximately 100 million times.
Pursuing research into superfluorescence through innovative experimental equipment and originality
This finding may lead to the development of quantum optical amplifiers in the future, and may also lead to further elucidation of the quantum world.
In fact, this research is not complete, and I believe there is an even bigger goal ahead. I want to shed light on the mysterious world of quantum mechanics. Quantum mechanics are extremely mysterious, and impossible phenomena can occur. The goal of this research is to unravel these secrets. One path to achieving this goal is research into superfluorescence. In the title of the paper published in the online version of the journal "Physical Review Letters," I write that I want to go as far as developing a quantum optical amplifier, and I think I'm being a little ambitious (laughs). That's how much of a worthwhile theme it is to pursue.
In fact, light that is highly quantum, in other words light that has quantum characteristics, has been developed using various technologies up to now. However, as far as I know, it is probably not possible to amplify the intensity of light while maintaining that state. Superfluorescence is an extremely special amplifier, so I thought it would be amazing if we could use this technology to amplify light, and this research was aimed at first clarifying whether this is possible or not.
If successful, it could lead to the development of quantum optical amplifiers in the future, and further down the line, it may be possible to use that light to unlock the secrets of quantum mechanics. I was willing to devote my entire research career to this, but I have now embarked on a long journey where no one has yet reached the goal. The results of this research represent a step up in the ladder that could potentially lead to the future.
First, I would like to explain the phenomenon of superfluorescence. This phenomenon was discovered by a researcher named R. Dicke in 1954, and was actively studied for a time several decades ago, but it is a research topic that has calmed down a bit recently. Superfluorescence is a phenomenon in which a group of excited atoms simultaneously emits fluorescence. When a material with pronounced quantum nature such as an atom (quantum material) is excited from a low-energy state to a high-energy state, its internal energy is converted into light and emitted as fluorescence into free space. When a large number of quantum materials are excited at the same time, each material interacts with each other, naturally aligning the timing of light emission, i.e., the phase, and emitting a light pulse with a high peak intensity different from general fluorescence. This is "superfluorescence". As a result of various verifications over the past half century, superfluorescence has been recognized as a universal phenomenon that can occur in any physical system.
In this study, we conducted an experiment to generate superfluorescence by irradiating an atomic ensemble with a weak laser beam that resonates with the wavelength of superfluorescence. As a result, we found that the phase of the laser beam was transferred to the phase of the superfluorescence, and we obtained experimental results that could be interpreted as the light intensity of the weak laser beam being coherently amplified by the superfluorescence (as if the wavelengths interfered with each other), and we found that the instantaneous intensity was actually amplified by seven orders of magnitude.
This phenomenon can be explained by the phenomenon of photon avalanche, in which the first photon emitted in superfluorescence primes the system and releases photons of the same phase one after another. The number of atoms synchronized in this experiment is estimated to be about 10⁸. In other words, a single photon primed the system and emitted a light pulse consisting of about 100 million photons. This demonstrates that superfluorescence will function as an extremely powerful light amplifier that amplifies the intensity of light in the future.
One of the reasons why such a thing has not been demonstrated in previous research on superfluorescence is that the experimental equipment has not yet evolved. After reaching its peak around 1980, various experimental equipment has evolved even during the period when superfluorescence research internationally waned somewhat. In this experiment, a pulsed laser device was used, which could only be controlled in units of 1 ns (nanosecond*), but nowadays, devices that can be controlled in units of 1/10,000 of that, or 100 fs (femtosecond*), are available commercially. In addition, the performance of continuous wave lasers has also evolved dramatically. Using these technologies, experiments that were previously impossible have become possible, and this time, by constructing an original device to demonstrate the amplification effect, we were able to derive experimental results. From this perspective, it is believed that the two catalysts that led to this experiment were the focus on the research field of superfluorescence, which at first glance was thought to have been exhausted, and the evolution of laser light source devices that allow us to delve deeper into that focus.
*1ns is <10 to the power of -9> seconds, 1fs is <10 to the power of -15> seconds
As we have discussed so far, superfluorescence itself has been a known phenomenon for a long time, but I believe that research into the quantum nature of it is now at the forefront of the world. Many researchers are beginning to feel that by utilizing superfluorescence to deepen research into quantum mechanisms, we may be able to gain new insights into the quantum world. With this background, I believe that the results of this experiment were published in the online version of the internationally acclaimed academic journal "Physical Review Letters."
Pursuing the quantum nature of superfluorescence not only allows us to approach the mysteries of quantum mechanics, but also leads to ideas about what quantum technologies can be developed in the future. We are still at the starting point of our research, and we need to identify various possibilities, such as "what will happen if we do this?" and "if this happens, then what about if we do this?" In that sense, I myself am very curious about future research in this field. Curiosity is different for each person, and I think there are people who are interested in various fields, but I have always had a strong interest in the "small world." In that sense, the quantum world is a world that stimulates intellectual curiosity.
If this were corporate research, we would be asked to produce output that would lead to business possibilities, but in the academic world, we can sit down and focus on our research. The students who will be working with me from now on will discover various technologies through their research, and if there are students among them who share their curiosity about the wonders of quantum mechanics, I think that this will be of the utmost value in terms of gaining value from their learning. You can think for yourself about what the quantum world is like, make a hypothesis, devise an experimental device, and see the results with your own eyes. Of course, classroom learning is important, but you can think for yourself through experiments, see with your own eyes, and think again at the end. I feel that our Faculty of Science and Engineering provides the perfect environment for students who are good at this.
The results of this research are limited to the light intensity, which can be measured by the ruler of classical physics. The synchrony of atomic groups can also only be explained by the theory of classical mechanics. On the other hand, since superfluorescence is originally a synchronization phenomenon in the world of quantum mechanics, we need to clarify how the quantum phenomenon of the amplification of laser light in superfluorescence differs from the phenomenon of classical mechanics. Specifically, our next goal is to set up a new device called cold atoms and observe the movement of atoms at extremely low temperatures, so that we can discuss the quantum nature of light.
I believe there will be many difficulties to overcome on the way to achieving this goal, but I expect that this will enable me to conduct even more interesting research than I am doing now.
Quantum has the characteristic of being entangled, where two quanta behave as a pair. As the name suggests, photon pairs refer to a state in which two photons have a quantum mechanical correlation. Various research studies around the world have already shown that in this quantum entangled state, observational results can be obtained that would not occur in classical mechanics. However, as in this research, no one has yet observed what quantum behavior is observed when a photon pair in a quantum entangled state is input to an atomic group that produces hyperfluorescence. In this area, we are considering precisely observing what quantum properties are retained in the light amplified this time.
In research, you don't always arrive at the data you want. When I started this research eight years ago, I had little knowledge of the phenomenon and was, so to speak, an outsider. From there, I analyzed many previous studies, tackled themes that other researchers were not interested in, and, through repeated trial and error while often unable to obtain clean data, accumulated small results, which led to this presentation.
After going through this process, when you finally get the clear experimental results that you had predicted in your hypothesis, it is an immense joy for you as a researcher and you immediately start thinking about what kind of interesting experiment you should do next.
I would also like all of you who are aspiring to enter the academic world to find something that you are passionate about. It doesn't have to be research. I myself took a long detour to find it, so I feel that the task of finding it is difficult, but I hope you will cherish your curiosity and dive into a world where you can find joy beyond your passion.